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Gamma Spectroscopy Analysis of Produced Water from Selected Flow Stations in Delta State, Nigeria

Received: 25 July 2013    Accepted:     Published: 10 September 2013
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Abstract

This paper present the findings of naturally occurring radionuclides (226Ra, 228Ra and 40K) carried out on produced water collected from seven oil and gas fields onshore of Delta State, using gamma spectroscopy. Twenty- one produced water samples from seven flow stations waste pit were collected within the oil fields using standard methods. The average specific activity concentrations for the radionuclides 40K, 226Ra and 228Ra are 48.7813.67Bql-1, 6.042.48Bql-1 and 5.182.14Bql-1 respectively. These obtained values are higher than the WHO, 2008 recommended standard limit of 10Bql-1, 1.0Bql-1 and 0.1Bql-1 for 40K, 226Ra and 228Ra respectively. Radium equivalent have average activity concentration of 14.365.55Bql-1 while the average absorbed dose rate of 6.68mSvy-1 was found to be higher than the UNSCEAR 2000 acceptable standard of 1.5mSvy-1. Although the hazard indices (Hex, Hin) calculated are still within their tolerable levels, the estimated committed effective dose due to intake of the sampled water for all the produced water considered are far above the ICRP 0.1 mSvyr-1 maximum permissible limit. The result indicates some level of water pollution in the studied water samples. This work will add to the world data base of natural radionuclide in produced water from crude oil.

Published in International Journal of Environmental Monitoring and Analysis (Volume 1, Issue 5)
DOI 10.11648/j.ijema.20130105.11
Page(s) 167-174
Creative Commons

This is an Open Access article, distributed under the terms of the Creative Commons Attribution 4.0 International License (http://creativecommons.org/licenses/by/4.0/), which permits unrestricted use, distribution and reproduction in any medium or format, provided the original work is properly cited.

Copyright

Copyright © The Author(s), 2024. Published by Science Publishing Group

Keywords

Natural Radioactivity, Produced Water, Oil Fields, Delta State

References
[1] Abbady A.G.E. 2004. Estimation of Radiation Hazard Indices from Sedimentary Rocks in Upper Egypt. Applied Radiation and Isotopes, 60: 111-114.
[2] Agbalagba E.O. and Onoja R.A., 2011. Evaluation of natural radioactivity in soil, sediment and water samples of Niger delta (Biseni) flood plain lakes, Nigeria. J. Environ. Rad. 102: 667-671
[3] Agbalagba, E.O., Avwiri, G.O. and Ononugbo, P.C. 2013. Activity concentration and radiological impact assessment of 226Ra, 228Ra and 40K in drinking waters from (OML) 30, 58 and 61 oil fields and host communities in Niger Delta region of Nigeria. Elsevier; Journal of Environmental Radioactivity116:197-200
[4] Ajayi O.S, and Achuka J (2009). Radioactivity in drilled and dug well drinking water of Ogun State Southwestern Nigeria and consequentdose estimates. Rad. Prot. Dos., 135(1) 54-63.
[5] Arogunjo, A.M., Ofuga, E.E. and Afolabi, M.A., 2005. Levels of natural radionuclides in some Nigerian cereals and tubers. J. Environ. Rad. 82:1- 6
[6] Avwiri, G.O. and Agbalagba, E.O. 2012. Studies on the radiological impact of oil and gas activities in Oil Mineral Lease 30 (OML3) oil fields in Delta State, Nigeria. J. Pet. Environ Biotechnol. 3(2): 1- 8.
[7] Beretka, I., Mathew, P.I., (1985). Natural radioactivity of Australian building materials, waste and by-products. Health Physics 48, 87–95.
[8] Chowdhurry, S., Husian, T., Veiteh, H., Bose, N. adna Sadiq, R., (2004): Human Health Risk Assessment of Naturally Occurring Radioactivity Materials in Produced Water, Canada.
[9] Diab, H. M., S.A. Nouh, A. Hamdy and S.A. El- Fiki, 2008. Evaluation of natural radioactivity in a cultivated area around a fertilizer factory. J. Nucl. and Rad. Phys. 3(1): 53- 62.
[10] Gafvert.T and Faerevik.I. 2004: Natural Radioactivity in Produced Water from Norwegian Oil and Gas Industry in 2003.
[11] IAEA (International Atomic Energy Agency), 2003. International Basic Safety Standards for protection against ionizing radiation and for the safety of radiation sources. No 115, (IAEA,Vienna 2003).
[12] ICRP (International Commission on Radiological Protection), 1997. ICRP Publication 78; Individual Monitoring for Internal Exposure of workers
[13] Isam-Salih, M.M., Pettersson, H.B. and Lund, E., 2002. Uranium and thorium series radionuclides in drinking water from drilled bedrock wells: correlation to geology and bedrock radioactivity and dose estimation. Radiat. Protect Dosim., 102(3), 249-258.
[14] Isehunwa S. O. and Onovae S., 2011. Evaluation of produced water discharge in the Niger-Delta. ARPN Journal of Engineering and Applied Sciences. VOL. 6, NO. 8, pg 66- 72. www.arpnjournals.com
[15] Ismail A.M., Kullab M.K. and Saq’an S.A, 2009. Natural radionuclides in bottled drinking water in Jordan and their committed effective doses. Jordan J. Phy.2(1):47-57
[16] Jerez Vegueria SF, Godoy JM, Miekeley N. 2002. Environmental impact studies of barium and radium discharges by produced water from the "Bacia de Campos" oil-field offshore platforms, Brazil. Journal of Environmental Radioactivity 2002; 62: 29-38.
[17] Neff JM (2002). Bioaccumulation in Marine Organisms; Effects of Contaminants from Oil Well Produced Water. pp Elsevier Science Ltd. Kidlington, Oxford, UK. pp 191-202.
[18] SPDC, EIA, 2004. Environmental impact assessment of Afiesere, Eriemu, Repele and Uzere for oil field development. Scooping workshop for EIA process, May 2004; pg 2-6.
[19] Strand T, Lysebo I, Kristensen D, Birovljev A., 1997. Deposits of naturally occurring radioactivity in production of oil and natural gas. NRPA report. Østerås, Norwegian Radiation Protection Authority Norwegian.
[20] Taiwo, B.A, and Akalia, T.C., 2009. Spatial variation in groundwater geochemistry and water quality index in Port Harcourt. Rivers State, Nigeria Scientia Africana 8(1): 134-155
[21] Tchokossa P, Olomo,J.B and Balogun, F.A., 2011. Assessment of Radionuclide Concentrations and Absorbed Dose from Consumption of Community Water Supplies in Oil and Gas Producing Areas in Delta State, Nigeria. World Journal of Nuclear Science and Technology, 1, 77-86
[22] Tchokosse, P., Olomo, J.B. and Osibota, O.A., 1999. Radioactivity in the community water supplies of Ife-central and Ife-East L.G.A.’S Osun State, Nigeria. Nucl. Instr. and Methods in Phys. Res. (A422:780-784).
[23] United Nations Scientific Committee on the Effects of Atomic Radiation (UNSCEAR), 2000. Sources and effects of ionizing radiation (Report to the General Assembly), New York: United Nation.
[24] UNSCEAR, 2000. Sources and Effects of Ionizing Radiation. United Nations Scientific Committee on the Effects of Atomic Radiation, United Nations, New York.
[25] Vegueria SFJ, Godoy JM and Miekeley N (2002). Environmental Impact in Sediments and Seawater due to Discharges of Ba,226Ra,228Ra, V, Ni, and Pb by Produced Water from the Bacia de Campos Oil Field Offshore Platforms; Environmental Forensics 3:115-123 .
[26] Vesterbacka Pia, 2007. Natural radioactivity in drinking water in Finland. Boreal Environ. Res. 12:11-16
[27] WHO, 2003. Guidelines for drinking water quality. Third ed., Radiological quality of drinking water, World Health Organization, Geneva, Switzerland.
[28] World Health Organization (WHO), 2008. Guidelines for drinking water policy 3rd ed., Incorporating the 1st and 2nd agenda, Vol.1 recommendation. WHO Geneva, Switzerland.
[29] Yusuf N.M., Hossian I. and Wagiran H., 2012. Natural radioactivity in drinking and Mineral Water. Scientific Research and Essays Vol. 7(9) pg. 1070-1075.
[30] Zarie, K.A. and K.S. Al Mugren, 2010. Measurement of natural radioactivity and assessment of radiation hazard in soil samples from Tayma area (KSA). Isotope and Rad. Res. 42(1):1-9.
Cite This Article
  • APA Style

    Avwiri Gregory O., Esi Emmanuel, Agbalagba Ezekiel O. (2013). Gamma Spectroscopy Analysis of Produced Water from Selected Flow Stations in Delta State, Nigeria. International Journal of Environmental Monitoring and Analysis, 1(5), 167-174. https://doi.org/10.11648/j.ijema.20130105.11

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    ACS Style

    Avwiri Gregory O.; Esi Emmanuel; Agbalagba Ezekiel O. Gamma Spectroscopy Analysis of Produced Water from Selected Flow Stations in Delta State, Nigeria. Int. J. Environ. Monit. Anal. 2013, 1(5), 167-174. doi: 10.11648/j.ijema.20130105.11

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    AMA Style

    Avwiri Gregory O., Esi Emmanuel, Agbalagba Ezekiel O. Gamma Spectroscopy Analysis of Produced Water from Selected Flow Stations in Delta State, Nigeria. Int J Environ Monit Anal. 2013;1(5):167-174. doi: 10.11648/j.ijema.20130105.11

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  • @article{10.11648/j.ijema.20130105.11,
      author = {Avwiri Gregory O. and Esi Emmanuel and Agbalagba Ezekiel O.},
      title = {Gamma Spectroscopy Analysis of Produced Water from Selected Flow Stations in Delta State, Nigeria},
      journal = {International Journal of Environmental Monitoring and Analysis},
      volume = {1},
      number = {5},
      pages = {167-174},
      doi = {10.11648/j.ijema.20130105.11},
      url = {https://doi.org/10.11648/j.ijema.20130105.11},
      eprint = {https://article.sciencepublishinggroup.com/pdf/10.11648.j.ijema.20130105.11},
      abstract = {This paper present the findings of naturally occurring radionuclides (226Ra, 228Ra and 40K) carried out on produced water collected from seven oil and gas fields onshore of Delta State, using gamma spectroscopy. Twenty- one produced water samples from seven flow stations waste pit were collected within the oil fields using standard methods. The average specific activity concentrations for the radionuclides 40K, 226Ra and 228Ra are 48.7813.67Bql-1, 6.042.48Bql-1 and 5.182.14Bql-1 respectively. These obtained values are higher than the WHO, 2008 recommended standard limit of 10Bql-1, 1.0Bql-1 and 0.1Bql-1 for 40K, 226Ra and 228Ra respectively. Radium equivalent have average activity concentration of 14.365.55Bql-1 while the average absorbed dose rate of 6.68mSvy-1 was found to be higher than the UNSCEAR 2000 acceptable standard of 1.5mSvy-1. Although the hazard indices (Hex, Hin) calculated are still within their tolerable levels, the estimated committed effective dose due to intake of the sampled water for all the produced water considered are far above the ICRP 0.1 mSvyr-1 maximum permissible limit. The result indicates some level of water pollution in the studied water samples. This work will add to the world data base of natural radionuclide in produced water from crude oil.},
     year = {2013}
    }
    

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  • TY  - JOUR
    T1  - Gamma Spectroscopy Analysis of Produced Water from Selected Flow Stations in Delta State, Nigeria
    AU  - Avwiri Gregory O.
    AU  - Esi Emmanuel
    AU  - Agbalagba Ezekiel O.
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    N1  - https://doi.org/10.11648/j.ijema.20130105.11
    DO  - 10.11648/j.ijema.20130105.11
    T2  - International Journal of Environmental Monitoring and Analysis
    JF  - International Journal of Environmental Monitoring and Analysis
    JO  - International Journal of Environmental Monitoring and Analysis
    SP  - 167
    EP  - 174
    PB  - Science Publishing Group
    SN  - 2328-7667
    UR  - https://doi.org/10.11648/j.ijema.20130105.11
    AB  - This paper present the findings of naturally occurring radionuclides (226Ra, 228Ra and 40K) carried out on produced water collected from seven oil and gas fields onshore of Delta State, using gamma spectroscopy. Twenty- one produced water samples from seven flow stations waste pit were collected within the oil fields using standard methods. The average specific activity concentrations for the radionuclides 40K, 226Ra and 228Ra are 48.7813.67Bql-1, 6.042.48Bql-1 and 5.182.14Bql-1 respectively. These obtained values are higher than the WHO, 2008 recommended standard limit of 10Bql-1, 1.0Bql-1 and 0.1Bql-1 for 40K, 226Ra and 228Ra respectively. Radium equivalent have average activity concentration of 14.365.55Bql-1 while the average absorbed dose rate of 6.68mSvy-1 was found to be higher than the UNSCEAR 2000 acceptable standard of 1.5mSvy-1. Although the hazard indices (Hex, Hin) calculated are still within their tolerable levels, the estimated committed effective dose due to intake of the sampled water for all the produced water considered are far above the ICRP 0.1 mSvyr-1 maximum permissible limit. The result indicates some level of water pollution in the studied water samples. This work will add to the world data base of natural radionuclide in produced water from crude oil.
    VL  - 1
    IS  - 5
    ER  - 

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Author Information
  • Department of Physics, University of Port Harcourt, Choba, Rivers State, Nigeria

  • Department of Physics, University of Port Harcourt, Choba, Rivers State, Nigeria

  • Department of Physics, Federal University of Petroleum Resources, Effurun, Nigeria

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