Characterization of Volatile Components of Eight FengHuang Dancong Manufactured Teas and Fresh Leaves by HS-SPME Coupled with GC-MS
International Journal of Nutrition and Food Sciences
Volume 7, Issue 5, September 2018, Pages: 160-172
Received: Aug. 15, 2018;
Accepted: Sep. 4, 2018;
Published: Oct. 9, 2018
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Jingfang Shi, Agro-Biological Gene Research Center, Guangdong Academy of Agricultural Sciences, Guangzhou, China
Wenjie Huang, Agro-Biological Gene Research Center, Guangdong Academy of Agricultural Sciences, Guangzhou, China
Zhuang Chen, Agro-Biological Gene Research Center, Guangdong Academy of Agricultural Sciences, Guangzhou, China
Shili Sun, Tea Research Institute, Guangdong Academy of Agricultural Sciences, Guangzhou, China
Limin Xiang, Tea Research Institute, Guangdong Academy of Agricultural Sciences, Guangzhou, China
Qian Kong, Agro-Biological Gene Research Center, Guangdong Academy of Agricultural Sciences, Guangzhou, China
Xiaohui Jiang, Tea Research Institute, Guangdong Academy of Agricultural Sciences, Guangzhou, China
Dong Chen, Tea Research Institute, Guangdong Academy of Agricultural Sciences, Guangzhou, China
Shijuan Yan, Agro-Biological Gene Research Center, Guangdong Academy of Agricultural Sciences, Guangzhou, China
FengHuang Dancong tea is famous for its excellent aroma quality. In order to characterize the volatile components in different aroma types of FengHuang Dancong tea, both fresh leaves and manufactured teas of seven well-known aroma types and their ancestor variety, which were harvested from the same places and manufactured using the same procedure, were investigated using headspace solid-phase microextraction (HS-SPME) coupled with gas chromatography-mass spectrometry (GC-MS). Results indicated that the volatile composition and contents of manufactured teas and fresh leaves, including HuangZhi, XingRen, GuiHua, MiLan, JiangHua, YuLan YeLai and Fenghuang Shuixian, were obviously different. Linalool, (E)-2-hexenal, cis-3-hexenyl acetate, linalool oxide, methyl salicylate, geraniol, and nerolidol were the major volatile components in fresh leaves, and their total relative contents ranged from 78.44-90.07%. But in manufactured teas, hotrienol, linalool, β-myrcene, D-limonene, 1-ethyl-1H-pyrrole-2-carboxaldehyde, β-ocimene, linalool oxide, benzyl nitrile, indole, jasmone, and nerolidol were the major volatile components, ranged from 60.12-93.97%. Although there were some similarities in the aroma composition and content among the manufactured teas of different aroma types, each type had unique aroma characteristics. The obvious difference between FengHuang Shuixian and other aroma types of manufactured teas may be due to the higher content of alkene and pyrrole derivatives and lower content of alcohols, especial terpene alcohols. Furthermore, the correlations between manufactured teas and the fresh leaves indicated that the volatile compounds profile of fresh leaves may affect the aroma quality of the manufactured tea. This study provided a comprehensive comparison of the volatile profile in different aroma types of Fenghuang Dancong tea, which is a scientific foundation for further quality assessment of Fenghuang Dancong variety in the future.
Characterization of Volatile Components of Eight FengHuang Dancong Manufactured Teas and Fresh Leaves by HS-SPME Coupled with GC-MS, International Journal of Nutrition and Food Sciences.
Vol. 7, No. 5,
2018, pp. 160-172.
Chen, Y. L., Duan, J., Jiang, Y. M., Shi, J., Peng, L., Xue, S., Kakuda, K. (2011). Production, quality, and biological effects of oolong tea (camellia sinensis). Food Reviews International, 27(1): 1-15.
Chen, Y. S., Tasy, H. R., Yu, T. H. (1998). Studies on the formation of special aroma compounds of Pouchung tea made from different varieties. Developments in Food Science, 40(98): 431-442.
Shi, M. N., Gong, S. Y. (2012). Research progress on tea aroma. Journal of Tea, 38(1): 19-23.
Ma, C., Qu, Y., Zhang, Y., Qiu, B., Wang, Y., Xi, C. (2014). Determination of nerolidol in teas using headspace solid phase microextraction-gas chromatography. Food Chemistry, 152(2): 285-290.
Dai, S., Xie, C., Li, Q., Chen, D., Zheng, R. (1998). Analysis on aromatic constituents of five well-known strains from fenghuang dancong tea cultivar. Journal of Tea Science, 18(1), 39-46
Rawat, R., Gulati, A., Kiranbabu, G., Acharya, R., Kaul, V., Singh, B. (2007). Characterization of volatile components of Kangra orthodox black tea by gas chromatography-mass spectrometry. Food Chemistry, 105 (1): 229-235.
Xu, Y. Q., Wang, C., Li, C. W., Liu, S. H., Zhang, C. X. Li, L. W. Jiang, D. H. (2015). Characterization of aroma-active compounds of pu-erh tea by headspace solid-phase microextraction (HS-SPME) and simultaneous distillation-extraction (SDE) coupled with GC-Olfactometry and GC-MS. Food Analytical Methods, 9(5): 1188-1198.
Xiao, Z., Wang, H., Niu, Y., Liu, Q., Zhu, J., Chen, H., Ma, N. (2017). Characterization of aroma compositions in different Chinese congou black teas using GC-MS and GC-O combined with partial least squares regression. Flavour and Fragrance Journal, 32(4): 265-276.
Gu, X., Zhang, Z., Wan, X,, Ning, J., Yao, C., Shao, W. (2009). Simultaneous distillation extraction of some volatile flavor components from pu-erh tea samples-comparison with steam distillation-liquid/liquid extraction and soxhlet extraction. International Journal of Analytical Chemistry, 276713.
Zhu, M., Li, E., He, H. (2008). Determination of volatile chemical constitutes in tea by simultaneous distillation extraction, vacuum hydrodistillation and thermal desorption. Chromatographia, 68 (7-8): 603-610.
Wu, Y., Lv, S., Lian, M., Wang, C., Gao, X., Meng, Q. (2016). Study of characteristic aroma components of baked Wujiatai green tea by HS-SPME/GC-MS combined with principal component analysis. CyTA-Journal of Food, 14(3): 423-432.
Mu, B., Zhu, Y., Lv, H. P., Yan, H., Peng, Q. H., Lin, Z. (2018). The enantiomeric distributions of volatile constituents in different tea cultivars. Food Chemistry, 265: 329-336.
Lv, S. D., Wu, Y. S., Jiang, Y. F., Meng, Q. X. (2014). Comparative analysis of aroma characteristics of oolong tea from different geographical regions. Food Science, 35(2): 146-153.
Yang, Z., Baldermann, S., Watanabe, N. (2013). Recent studies of the volatile compounds in tea. Food Research International, 53(2): 585-599.
Zheng, X. Q., Li, Q. S., Xiang, L. P., Liang, Y. R. (2016). Recent advances in volatiles of teas. Molecules, 21(3): 338.
Wang, C., Zhang, C., Kong, Y., Peng, X., Li, C., Liu, S., Du, L., Xiao, D., Xu, Y. (2017). A comparative study of volatile components in Dianhong teas from fresh leaves of four tea cultivars by using chromatography-mass spectrometry, multivariate data analysis, and descriptive sensory analysis. Food Research Intermational, 100(1): 267-275.
Pripdeevech, P., Machan. T. (2011). Fingerprint of volatile flavour constituents and antioxidant activities of teas from Thailand. Food Chemistry, 125(2): 797-802.
Katsuno, T., Kasuga, H., Kusano, Y., Yaguchi, Y., Tomomura, M., Cui, J., Yang, Z., Baldermann, S., Nakamura, Y., Ohnishi, T., Mase, N., Watanabe, N. (2014). Characterisation of odorant compounds and their biochemical formation in green tea with a low temperature storage process. Food Chemistry, 148(148C): 388-395.
Xu, X., Yan, M., Zhu, Y. (2005). Influence of fungal fermentation on the development of volatile compounds in the puer tea manufacturing process. Engineering in Life Sciences, 5(4): 382-386.
Zhu, J., Chen, F., Wang, L., Niu, Y., Yu, D., Shu, C., Chen, H., Wang, H., Xiao, Z. (2015). Comparison of aroma-active volatiles in oolong tea infusions using GC-Olfactometry, GC-FPD, and GC-MS. Journal of Agricultural and Food Chemistry, 63(34): 7499-7510.
Wang, B. S., Yu, H. M., Chang, L. W., Yen, W. J., Duh, P. D. (2008). Protective effects of pu-erh tea on LDL oxidation and nitric oxide generation in macrophage cells. LWT-Food Science and Technology, 41(6): 1122-1132.
Xiao, Z., Chen, H., Niu, Y., Wu, M., Chang, S., Zhu, J. (2015). Identify the characteristic aroma components of longjing tea by headspace steam distillation extraction and GC-MS/GC-O. Journal of Zhejiang University, 42(6): 714-720.
Wang, C., Lv, S., Wu, Y., Gao, X., Li, J., Zhang, W., Meng, Q. (2016). Oolong tea made from tea plants from different locations in Yunnan and Fujian, China showed similar aroma but different taste characteristics. Springerplus, 5(1): 576.
Alasalvar, C., Topal, B., Serpen, A., Bahar, B., Pelvan, E., Gokmen, V. (2012). Flavor characteristics of seven grades of black tea produced in Turkey. Journal of Agricultural and Food Chemistry, 60(25): 6323-6332.
Zhu, Y., Shao, C. Y., Lv, H. P., Zhang, Y., Dai, W. D., Guo, L., Tan, J. F., Peng, Q. H., Lin, Z. (2017). Enantiomeric and quantitative analysis of volatile terpenoids in different teas (Camellia sinensis). Journal of Chromatography A, 1490: 177-190.
Huang, D., Qi, D., Shen, C., Deng, Y., Wang, X., Li, Y. (2016). The preliminary study of fresh leaves aroma components of different oolong tea varieties. Chinese Agricultural Science Bulletin, 32(10): 189-199.
Ravichandran, R., Parthiban, R. (2000). Lipid occurrence, distribution and degradation to flavour volatiles during tea processing. Food Chemistry, 68(1): 7-13.
Zeng, L., Zhou, Y., Fu, X., Mei, X., Cheng, S., Gui, J., Dong, F., Tang, J., Ma, S., Yang, Z. (2017). Does oolong tea (Camellia sinensis) made from a combination of leaf and stem smell more aromatic than leaf-only tea? Contribution of the stem to oolong tea aroma. Food Chemistry, 237: 488-498.
Wang, L. F., Lee, J. Y., Chung, J. O., Baik, J. H., So, S., Park, S. K. (2008). Discrimination of teas with different degrees of fermentation by SPME-GC analysis of the characteristic volatile flavour compounds. Food Chemistry, 109(1): 196-206.
Zhou, C., Zhuang, D., Guo, S., Zhu, H., Ma, R.,Wu, Q. (2014). Classification and identification of different aromatics in tea made from different cultivar of Fenghuang Dancong. Journal of Tea Science, 34(6): 609-616.
Zhang, X., Tian, Y. E., Gao, F., Shi, B., Chen, R. (2015). Analysis of volatile compounds of Huangzhi aromatic Camellia sinensis cv. Fenghuangdancong tea. Farm Products Processing, 19.